A mathematical framework for the classification of
Self-assembling
Polypeptide Nanoparticles
Giuliana Indelicato, University of Torino
Abstract:
In the last decade scientists have started engineering many
different
self-assembling protein nanoparticles. The possible applications are
manifold and innovative: from vectors for the delivery of genes or
drugs to
synthetic vaccines. The fast development of this research field
poses new
challenges for the structural analysis as, in general, synthetic
nanoparticles do not fit into the Caspar and Klug’s framework: an
original
approach is needed to provide blueprints for the experimental
determination
of their structure.
We focus on a *de novo *class of proteins, referred to as
self-assembling
protein nanoparticles (SAPNs). This is a family of nanoparticles
that
provide a versatile platform for synthetic vaccines against a broad
range
of diseases, including malaria, SARS, influenza and HIV.
These nanoparticles self assemble from multiple copies of a
polypeptide
synthesized to have specific connectivity properties. The
polypeptides bind
to each other following precise local assembly rules, forming groups
of
five or three polypeptides. To elucidate the resulting assembled
global
structure, we use tools from graph theory. This approach unveils a
hidden
relation with fullerene geometries and enables a full classification
of the
high and low symmetry particles observed in experiments.